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In February 2007, Lee announced her new digital single which would essentially be the soundtrack to If in Love... She performed all three main tracks from the single on Inkigayo on February 25, 2007.The lead song was "Toc Toc Toc" (Korean: The single, although initially given a digital-only release, was given a limited retail release of only 30,000 copies.A music video was released for "Swing" (Korean: ; RR: Geune), featuring Gary from Leessang, on March 31, 2010.The lead single "Chitty Chitty Bang Bang" and its music video were released soon after.
An edited two-episode version of the drama also ran on SBS.
Upon release, tickets to the concert sold out in five minutes.
Her third studio album, It's Hyorish, was released on July 14, 2008.
The album has 14 tracks, including collaborations with Daesung from Big Bang, Jeon Ji-yoon from 4Minute, Bekah from After School, Gary from Leessang, and Sangchu from Mighty Mouth.
The singer worked also with E-Tribe, the team behind "U-Go-Girl", the lead single from her previous album.She also became an increasing presence in the civic community, emerging as one of the country's most high-profile animals rights activists.